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Electrochemical Switching with 3D DNA Tetrahedral Nanostructures Self-Assembled at Gold Electrodes | |
Abi, A; Lin, MH; Pei, H; Fan, CH; Ferapontova, EE; Zuo, XL; fchh@sinap.ac.cn; elena.ferapontova@inano.au.dk; zuoxiaolei@sinap.ac.cn | |
2014 | |
Source Publication | ACS APPLIED MATERIALS & INTERFACES
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ISSN | 1944-8244 |
Volume | 6Issue:11Pages:8928—8931 |
Abstract | Nanomechanical switching of functional three-dimensional (3D) DNA nanostructures is crucial for nanobiotechnological applications such as nanorobotics or self-regulating sensor and actuator devices. Here, DNA tetrahedral nanostructures self-assembled onto gold electrodes were shown to undergo the electronically addressable nanoswitching due to their mechanical reconfiguration upon external chemical stimuli. That enables construction of robust surface-tethered electronic nanodevices based on 3D DNA tetrahedra. One edge of the tetrahedron contained a partially self-complementary region with a stem-loop hairpin structure, reconfigurable upon hybridization to a complementary DNA (stimulus DNA) sequence. A non-intercalative ferrocene (Fc) redox label was attached to the reconfigurable tetrahedron edge in such a way that reconfiguration of this edge changed the distance between the electrode and Fc. |
Keyword | Transport Duplexes End Sensors |
Indexed By | SCI |
Language | 英语 |
WOS ID | WOS:000337336900117 |
Citation statistics | |
Document Type | 期刊论文 |
Identifier | http://ir.sinap.ac.cn/handle/331007/14113 |
Collection | 中科院上海应用物理研究所2011-2020年 |
Corresponding Author | fchh@sinap.ac.cn; elena.ferapontova@inano.au.dk; zuoxiaolei@sinap.ac.cn |
Recommended Citation GB/T 7714 | Abi, A,Lin, MH,Pei, H,et al. Electrochemical Switching with 3D DNA Tetrahedral Nanostructures Self-Assembled at Gold Electrodes[J]. ACS APPLIED MATERIALS & INTERFACES,2014,6(11):8928—8931. |
APA | Abi, A.,Lin, MH.,Pei, H.,Fan, CH.,Ferapontova, EE.,...&zuoxiaolei@sinap.ac.cn.(2014).Electrochemical Switching with 3D DNA Tetrahedral Nanostructures Self-Assembled at Gold Electrodes.ACS APPLIED MATERIALS & INTERFACES,6(11),8928—8931. |
MLA | Abi, A,et al."Electrochemical Switching with 3D DNA Tetrahedral Nanostructures Self-Assembled at Gold Electrodes".ACS APPLIED MATERIALS & INTERFACES 6.11(2014):8928—8931. |
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