CAS OpenIR  > 中科院上海应用物理研究所2011-2019年
Nitrogen-doped graphene supported Pd@PdO core-shell clusters for C-C coupling reactions
Jiang, BJ; Song, SZ; Wang, JQ; Xie, Y; Chu, WY; Li, HF; Xu, H; Tian, CG; Fu, HG; fuhg@vip.sina.com
2014
Source PublicationNANO RESEARCH
ISSN1998-0124
Volume7Issue:9Pages:1280—1290
AbstractThe introduction of nitrogen significantly decreases the metal particle size and improves the performance of metal-based graphene-supported catalysts. In this work, the density functional theory is used to understand the interaction between nitrogen-doped graphene and Pd@PdO clusters. Experiments show that small size Pd@PdO clusters (1-2 nm) can be grown uniformly on nitrogen-doped graphene sheets by a facile oxidation-reduction method. The nanoscale interaction relationship between nitrogen-doped graphene and Pd@PdO clusters is investigated through X-ray photoelectron spectroscopy (XPS) and X-ray absorption spectra (XAS). The composite catalysts are applied in Suzuki-Miyaura reactions giving high yields and good structural stability. These results have potential impact in design and optimization of future high performance catalyst materials for cross coupling reactions.
KeywordEnhanced Photocatalytic Activity Ray-absorption Spectroscopy Palladium Nanoparticles Graphite Oxide Catalyst Fabrication Reduction Resonance Facets Growth
Indexed BySCI
Language英语
WOS IDWOS:000342080100005
Citation statistics
Cited Times:46[WOS]   [WOS Record]     [Related Records in WOS]
Document Type期刊论文
Identifierhttp://ir.sinap.ac.cn/handle/331007/14274
Collection中科院上海应用物理研究所2011-2019年
Corresponding Authorfuhg@vip.sina.com
Recommended Citation
GB/T 7714
Jiang, BJ,Song, SZ,Wang, JQ,et al. Nitrogen-doped graphene supported Pd@PdO core-shell clusters for C-C coupling reactions[J]. NANO RESEARCH,2014,7(9):1280—1290.
APA Jiang, BJ.,Song, SZ.,Wang, JQ.,Xie, Y.,Chu, WY.,...&fuhg@vip.sina.com.(2014).Nitrogen-doped graphene supported Pd@PdO core-shell clusters for C-C coupling reactions.NANO RESEARCH,7(9),1280—1290.
MLA Jiang, BJ,et al."Nitrogen-doped graphene supported Pd@PdO core-shell clusters for C-C coupling reactions".NANO RESEARCH 7.9(2014):1280—1290.
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