Structural Phase Transitions and Metallized Phenomena in Arsenic Telluride under High Pressure
Zhao, JG; Yang, LX; Yu, ZH; Wang, Y; Li, CY; Yang, K; Liu, ZG; Wang, Y; Wang, Y (reprint author), Harbin Inst Technol, Acad Fundamental & Interdisciplinary Sci, Nat Sci Res Ctr, Harbin 150080, Peoples R China.; Liu, ZG (reprint author), Harbin Inst Technol, Dept Phys, Harbin 150080, Peoples R China.
2016
发表期刊INORGANIC CHEMISTRY
ISSN0020-1669
卷号55期号:8页码:3907—3914
文章类型期刊文献
摘要In this study, first-principle,calculations, in situ angle-dispersive X-ray diffraction, and in situ electrical resistance measurements were performed on arsenic telluride (As2Te3) under high pressure. Structural phase transitions and metallized phenomena were observed from the calculated and experimental results. Upon compression, alpha-As2Te3 transforms into phases alpha' and alpha '' at similar to 5.09 and similar to 13.2 GPa, respectively, with two isostructural phase transitions. From 13.2 GPa, As2Te3 starts to transform into phase gamma, with one first-order monoclinic to monoclinic crystal structural phase transition. According to the first-principle calculations and electrical resistance measurements, the structural phase transitions in the compression process induce the transformation from an insulator (phase alpha) across a semimetal (phase alpha') into a metal (phases alpha '' and gamma). The evolution of the structure and transport property upon compression on As2Te3 is helpful for understanding the properties of other A(2)B(3)-type compounds under high, pressure.
关键词Topological Insulator Crystal Structure Sb2te3 Bi2te3 As2te3 Refinement Bcc Superconductivity Polymorphism Beta-as2te3
DOI10.1021/acs.inorgchem.6b00073
收录类别SCI
语种英语
WOS记录号WOS:000374508600024
引用统计
被引频次:8[WOS]   [WOS记录]     [WOS相关记录]
文献类型期刊论文
条目标识符http://ir.sinap.ac.cn/handle/331007/25845
专题中科院上海应用物理研究所2011-2018年
通讯作者Zhao, JG; Wang, Y (reprint author), Harbin Inst Technol, Acad Fundamental & Interdisciplinary Sci, Nat Sci Res Ctr, Harbin 150080, Peoples R China.; Liu, ZG (reprint author), Harbin Inst Technol, Dept Phys, Harbin 150080, Peoples R China.
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Zhao, JG,Yang, LX,Yu, ZH,et al. Structural Phase Transitions and Metallized Phenomena in Arsenic Telluride under High Pressure[J]. INORGANIC CHEMISTRY,2016,55(8):3907—3914.
APA Zhao, JG.,Yang, LX.,Yu, ZH.,Wang, Y.,Li, CY.,...&Liu, ZG .(2016).Structural Phase Transitions and Metallized Phenomena in Arsenic Telluride under High Pressure.INORGANIC CHEMISTRY,55(8),3907—3914.
MLA Zhao, JG,et al."Structural Phase Transitions and Metallized Phenomena in Arsenic Telluride under High Pressure".INORGANIC CHEMISTRY 55.8(2016):3907—3914.
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