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Unveiling Microscopic Structures of Charged Water Interfaces by Surface-Specific Vibrational Spectroscopy
Wen, YC; Zha, S; Liu, X; Yang, SS; Guo, P; Shi, GS; Fang, HP; Shen, YR; Tian, CS; Shen, YR (reprint author), Fudan Univ, Dept Phys, State Key Lab Surface Phys, Shanghai 200433, Peoples R China.
2016
Source PublicationPHYSICAL REVIEW LETTERS
ISSN0031-9007
Volume116Issue:1Pages:
Subtype期刊文献
AbstractA sum-frequency spectroscopy scheme is developed that allows the measurement of vibrational spectra of the interfacial molecular structure of charged water interfaces. The application of this scheme to a prototype lipid-aqueous interface as a demonstration reveals an interfacial hydrogen-bonding water layer structure that responds sensitively to the charge state of the lipid headgroup and its interaction with specific ions. This novel technique provides unique opportunities to search for better understanding of electrochemistry and biological aqueous interfaces at a deeper molecular level.
KeywordSum-frequency Generation X-ray-diffraction Absorption Spectroscopy Atomic-resolution Aqueous-solutions Acid Monolayers Molecules Polarization Carboxylate Potentials
DOI10.1103/PhysRevLett.116.016101
Indexed BySCI
Language英语
WOS IDWOS:000367677300003
Citation statistics
Document Type期刊论文
Identifierhttp://ir.sinap.ac.cn/handle/331007/25887
Collection中科院上海应用物理研究所2011-2018年
Corresponding AuthorShen, YR (reprint author), Fudan Univ, Dept Phys, State Key Lab Surface Phys, Shanghai 200433, Peoples R China.
Recommended Citation
GB/T 7714
Wen, YC,Zha, S,Liu, X,et al. Unveiling Microscopic Structures of Charged Water Interfaces by Surface-Specific Vibrational Spectroscopy[J]. PHYSICAL REVIEW LETTERS,2016,116(1):—.
APA Wen, YC.,Zha, S.,Liu, X.,Yang, SS.,Guo, P.,...&Shen, YR .(2016).Unveiling Microscopic Structures of Charged Water Interfaces by Surface-Specific Vibrational Spectroscopy.PHYSICAL REVIEW LETTERS,116(1),—.
MLA Wen, YC,et al."Unveiling Microscopic Structures of Charged Water Interfaces by Surface-Specific Vibrational Spectroscopy".PHYSICAL REVIEW LETTERS 116.1(2016):—.
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