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Exploring the working mechanism of Li+ in O3-type NaLi0.1Ni0.35Mn0.55O2 cathode materials for rechargeable Na-ion batteries
Zheng, SY; Zhong, GM; McDonald, MJ; Gong, ZL; Liu, R; Wen, W; Yang, C; Yang, Y; Yang, Y (reprint author), Xiamen Univ, Collaborat Innovat Ctr Chem Energy Mat, State Key Lab Phys Chem Solid Surface, Dept Chem,Coll Chem & Chem Engn, Xiamen 361005, Peoples R China.; Yang, Y (reprint author), Xiamen Univ, Sch Energy Res, Xiamen 361005, Peoples R China.
2016
Source PublicationJOURNAL OF MATERIALS CHEMISTRY A
ISSN2050-7488
Volume4Issue:23Pages:9054-9062
Subtype期刊论文
AbstractNa-ion batteries (NIBs) have recently attracted much attention, due to their low cost and the abundance of sodium resources. In this work, NaLi0.1Ni0.35Mn0.55O2 as a promising new kind of cathode material for Na-ion batteries was synthesized by a co-precipitation method. Powder XRD patterns show that the sample has a primary O3-type structure after Li+ substitution. The material delivers excellent electrochemical performance, with an initial discharge specific capacity of 128 mA h g(-1) and a capacity retention of 85% after 100 cycles at a rate of 12 mA g(-1) in the voltage range of 2.0-4.2 V. In a widened voltage range of 1.5-4.3 V, the specific capacity can reach up to 160 mA h g(-1). The structural stability of the material is substantially improved compared with lithium-free NaNi0.5Mn0.5O2, which can be attributed to the formation of an O'3 phase caused by Li-substitution, as proven by in situ XRD and solid state NMR (ss-NMR) measurements.
DOI10.1039/c6ta02230h
Indexed BySCI
Language英语
WOS IDWOS:000378947200016
Citation statistics
Cited Times:26[WOS]   [WOS Record]     [Related Records in WOS]
Document Type期刊论文
Identifierhttp://ir.sinap.ac.cn/handle/331007/26503
Collection中科院上海应用物理研究所2011-2018年
Corresponding AuthorYang, Y (reprint author), Xiamen Univ, Collaborat Innovat Ctr Chem Energy Mat, State Key Lab Phys Chem Solid Surface, Dept Chem,Coll Chem & Chem Engn, Xiamen 361005, Peoples R China.; Yang, Y (reprint author), Xiamen Univ, Sch Energy Res, Xiamen 361005, Peoples R China.
Recommended Citation
GB/T 7714
Zheng, SY,Zhong, GM,McDonald, MJ,et al. Exploring the working mechanism of Li+ in O3-type NaLi0.1Ni0.35Mn0.55O2 cathode materials for rechargeable Na-ion batteries[J]. JOURNAL OF MATERIALS CHEMISTRY A,2016,4(23):9054-9062.
APA Zheng, SY.,Zhong, GM.,McDonald, MJ.,Gong, ZL.,Liu, R.,...&Yang, Y .(2016).Exploring the working mechanism of Li+ in O3-type NaLi0.1Ni0.35Mn0.55O2 cathode materials for rechargeable Na-ion batteries.JOURNAL OF MATERIALS CHEMISTRY A,4(23),9054-9062.
MLA Zheng, SY,et al."Exploring the working mechanism of Li+ in O3-type NaLi0.1Ni0.35Mn0.55O2 cathode materials for rechargeable Na-ion batteries".JOURNAL OF MATERIALS CHEMISTRY A 4.23(2016):9054-9062.
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