Nanobubbles at Hydrophilic Particle-Water Interfaces

doi:10.1021/acs.langmuir.6b01483

CAS OpenIR > 中科院上海应用物理研究所2011-2018年

	Nanobubbles at Hydrophilic Particle-Water Interfaces
	Pan, G; He, GZ; Zhang, MY; Zhou, Q; Tyliszczak, T; Tai, RZ; Guo, JH; Bi, L; Wang, L; Zhang, HG; Pan, G (reprint author), Chinese Acad Sci, Ecoenvironm Sci Res Ctr, Beijing 100085, Peoples R China.; Pan, G (reprint author), Nottingham Trent Univ, Sch Anim Rural & Environm Sci, Brackenhurst Campus, Southwell NG25 0QF, England.
	2016
发表期刊	LANGMUIR
ISSN	0743-7463
卷号	32 期号:43 页码:11133-11137
文章类型	期刊论文
摘要	The puzzling persistence of nanobubbles breaks Laplaces law for bubbles, which is of great interest for promising applications in surface processing, H-2 and CO2 storage, water treatment, and drug delivery. So far, nanobubbles have mostly been reported on hydrophobic planar substrates with atomic flatness. It remains a challenge to quantify nanobubbles on rough and irregular surfaces because of the lack of a characterization technique that can detect both the nanobubble morphology and chemical composition inside individual nanobubble-like objects. Here, by using synchrotron-based scanning transmission soft X-ray microscopy (STXM) with nanometer resolution, we discern nanoscopic gas bubbles of >25 nm with direct in situ proof of O-2 inside the nanobubbles at a hydrophilic particle-water interface under ambient conditions. We find a stable cloud of O-2 nanobubbles at the diatomite particle-water interface hours after oxygen aeration and temperature variation. The in situ technique may be useful for many surface nanobubble-related studies such as material preparation and property manipulation, phase equilibrium, nucleation kinetics, and relationships with chemical composition within the confined nanoscale space. The oxygen nanobubble clouds may be important in modifying particle-water interfaces and offering breakthrough technologies for oxygen delivery in sediment and/or deep water environments.
DOI	10.1021/acs.langmuir.6b01483
收录类别	SCI
语种	英语
WOS记录号	WOS:000386991700008
引用统计	被引频次：5[WOS] [WOS记录] [WOS相关记录]
文献类型	期刊论文
条目标识符	http://ir.sinap.ac.cn/handle/331007/26581
专题	中科院上海应用物理研究所2011-2018年
通讯作者	Pan, G (reprint author), Chinese Acad Sci, Ecoenvironm Sci Res Ctr, Beijing 100085, Peoples R China.; Pan, G (reprint author), Nottingham Trent Univ, Sch Anim Rural & Environm Sci, Brackenhurst Campus, Southwell NG25 0QF, England.
推荐引用方式 GB/T 7714	Pan, G,He, GZ,Zhang, MY,et al. Nanobubbles at Hydrophilic Particle-Water Interfaces[J]. LANGMUIR,2016,32(43):11133-11137.
APA	Pan, G.,He, GZ.,Zhang, MY.,Zhou, Q.,Tyliszczak, T.,...&Pan, G .(2016).Nanobubbles at Hydrophilic Particle-Water Interfaces.LANGMUIR,32(43),11133-11137.
MLA	Pan, G,et al."Nanobubbles at Hydrophilic Particle-Water Interfaces".LANGMUIR 32.43(2016):11133-11137.

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文件名称/大小	文献类型	版本类型	开放类型	使用许可
Nanobubbles at Hydro（1273KB）	期刊论文	作者接受稿	开放获取	CC BY-NC-SA	请求全文