Radiolysis products and degradation mechanism studies on tri-isoamyl phosphate (TiAP)
Li, RF; Cao, XJ; Zhao, HG; Liu, CX; Li, Z; Wang, JH; Zhang, L; Li, QG
2018
发表期刊RADIOCHIMICA ACTA
ISSN0033-8230
卷号106期号:3页码:239-247
文章类型期刊论文
摘要As an alternate extractant for spent fuel reprocessing, the radiolysis properties of TiAP should be systematically studied to evaluate the feasibility of using it in engineering scale. In this paper, the irradiation stability of TiAP was investigated by using the concept of radiolysis ratio and G value. It is found the extent of radiolysis would be increased with the increasing of absorbed doses, but decreased with the increasing of pre-equilibrium aqueous HNO3 concentration. Furthermore, the radiolysis products were analyzed qualitatively and quantitatively with gas, liquid and ion chromatograph, based on which the possible radiolysis mechanism of TiAP was also concluded.
关键词3rd Phase-formation Dodecane-tributylphosphate Solutions Tributyl-phosphate Solvent-extraction Purex Process Separation Systems Actinides Diluent u(Vi)
DOI10.1515/ract-2017-2803
收录类别SCI
语种英语
WOS记录号WOS:000425945100007
引用统计
文献类型期刊论文
条目标识符http://ir.sinap.ac.cn/handle/331007/29119
专题中科院上海应用物理研究所2011-2018年
作者单位1.Li, RF
2.Cao, XJ
3.Zhao, HG
4.Liu, CX
5.Li, Z
6.Wang, JH
7.Zhang, L
8.Li, QG
推荐引用方式
GB/T 7714
Li, RF,Cao, XJ,Zhao, HG,et al. Radiolysis products and degradation mechanism studies on tri-isoamyl phosphate (TiAP)[J]. RADIOCHIMICA ACTA,2018,106(3):239-247.
APA Li, RF.,Cao, XJ.,Zhao, HG.,Liu, CX.,Li, Z.,...&Li, QG.(2018).Radiolysis products and degradation mechanism studies on tri-isoamyl phosphate (TiAP).RADIOCHIMICA ACTA,106(3),239-247.
MLA Li, RF,et al."Radiolysis products and degradation mechanism studies on tri-isoamyl phosphate (TiAP)".RADIOCHIMICA ACTA 106.3(2018):239-247.
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