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Role of local structure distortion in the suppression of superconductivity for Eu3-xSrxBi2S4F4 system
Cheng, J; Zhang, P; Dong, P; Wang, XF; Wang, Y; Li, X; Liu, SL; Li, YK; Xu, Z
2018
Source PublicationJOURNAL OF ALLOYS AND COMPOUNDS
ISSN0925-8388
Volume743Pages:547-552
Subtype期刊论文
AbstractAs new family of superconductors with a layered structure, BiS2-based materials have attracted much interest. Eu3Bi2S4F4 is a newly discovered member which shows superconductivity at 1.5 K without extrinsic doping, however, superconductivity is strongly suppressed by Sr-doping. In this contribution, we present, in terms of local atomic displacement, an insight into the relationship between Sr-doping and the suppression of superconductivity in Eu3-xSrxBi2S4F4 by Bi and Eu L-3-edge X-ray absorption spectroscopy. Upon Sr-doping, the distance between Eu3F4 blocking layers and BiS2 layers is significantly elongated, accompanied by the breaking of Eu-S-Bi channel, which makes it more difficult to transfer electrons into BiS2 layers. Moreover, distortions in the Bi-S-1 plane increase with Sr content, reducing the overlap among Bi(6p(x)/6p(y))-S(3p) orbitals within the superconducting plane. The decoupling between blocking and BiS2 layers, as well as the distortions in the superconducting Bi-S-1 plane, may contribute to the suppression of superconductivity in Sr-doped Eu3Bi2S4F4 compounds. (C) 2018 Elsevier B.V. All rights reserved.
KeywordRay-absorption Spectroscopy Near-edge Structure Liii-absorption Valence Eu
DOI10.1016/j.jallcom.2018.01.410
Indexed BySCI
Language英语
WOS IDWOS:000427511200062
Citation statistics
Cited Times:5[WOS]   [WOS Record]     [Related Records in WOS]
Document Type期刊论文
Identifierhttp://ir.sinap.ac.cn/handle/331007/29124
Collection中科院上海应用物理研究所2011-2019年
Affiliation1.Cheng, J
2.Zhang, P
3.Dong, P
4.Wang, XF
5.Wang, Y
6.Li, X
7.Liu, SL
8.Li, YK
9.Xu, Z
Recommended Citation
GB/T 7714
Cheng, J,Zhang, P,Dong, P,et al. Role of local structure distortion in the suppression of superconductivity for Eu3-xSrxBi2S4F4 system[J]. JOURNAL OF ALLOYS AND COMPOUNDS,2018,743:547-552.
APA Cheng, J.,Zhang, P.,Dong, P.,Wang, XF.,Wang, Y.,...&Xu, Z.(2018).Role of local structure distortion in the suppression of superconductivity for Eu3-xSrxBi2S4F4 system.JOURNAL OF ALLOYS AND COMPOUNDS,743,547-552.
MLA Cheng, J,et al."Role of local structure distortion in the suppression of superconductivity for Eu3-xSrxBi2S4F4 system".JOURNAL OF ALLOYS AND COMPOUNDS 743(2018):547-552.
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