X-ray absorption spectroscopy study of synthetic cobalt blue pigments similar to Kangxi blue and white porcelain
Luo, M; Zhang, ML; Yan, WS; Wang, LH; Jiang, Z
2018
发表期刊JOURNAL OF THE AMERICAN CERAMIC SOCIETY
ISSN0002-7820
卷号101期号:5页码:2130-2136
文章类型期刊论文
摘要A series of cobalt blue pigments, which were synthesized based on the chemical compositions of the blue pigments in Kangxi blue and white porcelain, were investigated by Co, Mn, and Fe K-edge and L-2,L-3-edge X-ray absorption spectroscopy to determine the oxidation states and species of the elements and to discern their impact on the blue color. The results reveal that Co is bivalent and mainly located at tetrahedral sites, which is the main parameter controlling the blue color. Mn is mainly present as Mn2+, or CoxZn1-xAl2O4 and Fe is mainly present as Fe3+. In particular, Fe3+ substitutes the Al in CoAl2O4 and occupies octahedral sites with a high Mn content. All the synthetic cobalt blue pigments can form a solid solution with various end-members or an intermediate solution spinel. The spectroscopic determination of the oxidation states and speciation of Co, Mn, and Fe furthers understanding of the coloration of blue pigments in blue and white porcelain.
关键词Fine-structure Co Speciation Alumina Microstructure Jingdezhen Dynasties Catalysts Glasses Yuan
DOI10.1111/jace.15353
收录类别SCI
语种英语
WOS记录号WOS:000426513900038
引用统计
文献类型期刊论文
条目标识符http://ir.sinap.ac.cn/handle/331007/29210
专题中科院上海应用物理研究所2011-2018年
作者单位1.Luo, M
2.Zhang, ML
3.Yan, WS
4.Wang, LH
5.Jiang, Z
推荐引用方式
GB/T 7714
Luo, M,Zhang, ML,Yan, WS,et al. X-ray absorption spectroscopy study of synthetic cobalt blue pigments similar to Kangxi blue and white porcelain[J]. JOURNAL OF THE AMERICAN CERAMIC SOCIETY,2018,101(5):2130-2136.
APA Luo, M,Zhang, ML,Yan, WS,Wang, LH,&Jiang, Z.(2018).X-ray absorption spectroscopy study of synthetic cobalt blue pigments similar to Kangxi blue and white porcelain.JOURNAL OF THE AMERICAN CERAMIC SOCIETY,101(5),2130-2136.
MLA Luo, M,et al."X-ray absorption spectroscopy study of synthetic cobalt blue pigments similar to Kangxi blue and white porcelain".JOURNAL OF THE AMERICAN CERAMIC SOCIETY 101.5(2018):2130-2136.
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