CAS OpenIR  > 中科院上海应用物理研究所2011-2020年
Boosting fast energy storage by synergistic engineering of carbon and deficiency
Deng, SJ; Zhu, H; Wang, GZ; Luo, M; Shen, SH; Ai, CZ; Yang, L; Lin, SW; Zhang, QH; Gu, L; Liu, B; Zhang, Y; Liu, Q; Pan, GX; Xiong, QQ; Wang, XL; Xia, XH; Tu, JP
2020
Source PublicationNATURE COMMUNICATIONS
ISSN2041-1723
Volume11Issue:1Pages:-
Subtype期刊论文
AbstractExploring advanced battery materials with fast charging/discharging capability is of great significance to the development of modern electric transportation. Herein we report a powerful synergistic engineering of carbon and deficiency to construct high-quality three/two-dimensional cross-linked Ti2Nb10O29-x@C composites at primary grain level with conformal and thickness-adjustable boundary carbon. Such exquisite boundary architecture is demonstrated to be capable of regulating the mechanical stress and concentration of oxygen deficiency for desired performance. Consequently, significantly improved electronic conductivity and enlarged lithium ion diffusion path, shortened activation process and better structural stability are realized in the designed Ti2Nb10O29-x@C composites. The optimized Ti2Nb10O29-x@C composite electrode shows fast charging/discharging capability with a high capacity of 197 mA h g(-1) at 20C (similar to 3 min) and excellent long-term durability with 98.7% electron and Li capacity retention over 500 cycles. Most importantly, the greatest applicability of our approach has been demonstrated by various other metal oxides, with tunable morphology, structure and composition.
KeywordLITHIUM-ION BATTERIES LONG-LIFE ANODE TI2NB10O29 OXIDE COMPOSITE SKELETON ARRAYS OXYGEN XANES
DOI10.1038/s41467-019-13945-1
Indexed BySCI
Language英语
Citation statistics
Cited Times:51[WOS]   [WOS Record]     [Related Records in WOS]
Document Type期刊论文
Identifierhttp://ir.sinap.ac.cn/handle/331007/32733
Collection中科院上海应用物理研究所2011-2020年
Affiliation1.Zhejiang Univ, State Key Lab Silicon Mat, Key Lab Adv Mat & Applicat Batteries Zhejiang Pro, Hangzhou 310027, Peoples R China
2.Zhejiang Univ, Sch Mat Sci & Engn, Hangzhou 310027, Peoples R China
3.City Univ Hong Kong, Dept Phys, Hong Kong 999077, Peoples R China
4.Hainan Univ, State Key Lab Marine Resource Utilizat South Chin, Haikou 570228, Hainan, Peoples R China
5.Chinese Acad Sci, Shanghai Inst Appl Phys, Shanghai Synchrotron Radiat Facil, Shanghai 201210, Peoples R China
6.Chinese Acad Sci, Inst Phys, Beijing 100190, Peoples R China
7.City Univ Hong Kong, Shenzhen Res Inst, Shenzhen 518057, Peoples R China
8.Huzhou Univ, Dept Chem Mat, Huzhou 313000, Peoples R China
9.Hangzhou Dianzi Univ, Coll Mat & Environm Engn, Hangzhou 310018, Zhejiang, Peoples R China
Recommended Citation
GB/T 7714
Deng, SJ,Zhu, H,Wang, GZ,et al. Boosting fast energy storage by synergistic engineering of carbon and deficiency[J]. NATURE COMMUNICATIONS,2020,11(1):-.
APA Deng, SJ.,Zhu, H.,Wang, GZ.,Luo, M.,Shen, SH.,...&Tu, JP.(2020).Boosting fast energy storage by synergistic engineering of carbon and deficiency.NATURE COMMUNICATIONS,11(1),-.
MLA Deng, SJ,et al."Boosting fast energy storage by synergistic engineering of carbon and deficiency".NATURE COMMUNICATIONS 11.1(2020):-.
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