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Embedded Nickel-Mesh Transparent Electrodes for Highly Efficient and Mechanically Stable Flexible Perovskite Photovoltaics: Toward a Portable Mobile Energy Source
Li, M; Zuo, WW; Ricciardulli, AG; Yang, YG; Liu, YH; Wang, Q; Wang, KL; Li, GX; Saliba, M; Di Girolamo, D; Abate, A; Wang, ZK
2020
Source PublicationADVANCED MATERIALS
ISSN0935-9648
Volume32Issue:38Pages:-
Subtype期刊论文
AbstractThe rapid development of Internet of Things mobile terminals has accelerated the market's demand for portable mobile power supplies and flexible wearable devices. Here, an embedded metal-mesh transparent conductive electrode (TCE) is prepared on poly(ethylene terephthalate) (PET) using a novel selective electrodeposition process combined with inverted film-processing methods. This embedded nickel (Ni)-mesh flexible TCE shows excellent photoelectric performance (sheet resistance of approximate to 0.2-0.5 omega sq(-1)at high transmittance of approximate to 85-87%) and mechanical durability. The PET/Ni-mesh/polymer poly(3,4-ethylenedioxythiophene):poly(styrenesulfonate) (PEDOT:PSS PH1000) hybrid electrode is used as a transparent electrode for perovskite solar cells (PSCs), which exhibit excellent electric properties and remarkable environmental and mechanical stability. A power conversion efficiency of 17.3% is obtained, which is the highest efficiency for a PSC based on flexible transparent metal electrodes to date. For perovskite crystals that require harsh growth conditions, their mechanical stability and environmental stability on flexible transparent embedded metal substrates are studied and improved. The resulting flexible device retains 76% of the original efficiency after 2000 bending cycles. The results of this work provide a step improvement in flexible PSCs.
KeywordSOLAR-CELLS GRAPHENE FILMS
DOI10.1002/adma.202003422
Indexed BySCI
Language英语
Citation statistics
Document Type期刊论文
Identifierhttp://ir.sinap.ac.cn/handle/331007/32845
Collection中科院上海应用物理研究所2011-2020年
Affiliation1.Soochow Univ, Inst Funct Nano & Soft Mat FUNSOM, Jiangsu Key Lab Carbon Based Funct Mat & Devices, Suzhou 215123, Peoples R China
2.Helmholtz Zentrum Berlin Mat & Energie, Kekulestr 5, D-12489 Berlin, Germany
3.Soochow Univ, Coll Chem Chem Engn & Mat Sci, Lab Adv Optoelect Mat, Suzhou 215123, Peoples R China
4.Tech Univ Darmstadt, Inst Mat Sci, Alarich Weiss Str 2, D-64287 Darmstadt, Germany
5.Chinese Acad Sci, Shanghai Adv Res Inst, Shanghai Inst Appl Phys, Shanghai Synchrotron Radiat Facil SSRF, 239 Zhangheng Rd, Shanghai 201204, Peoples R China
6.Soochow Univ, Sch Optoelect Sci & Engn, Key Lab Adv Opt Mfg Technol Jiangsu Prov, Key Lab Modern Opt Technol Educ Minist China, Suzhou 215123, Peoples R China
7.Forschungszentrum Julich, IEK5 Photovolta, Helmholtz Young Investigator Grp, D-52425 Julich, Germany
8.Univ Naples Federico II, Dept Chem Mat & Prod Engn, Piazzale Tecchio 80, I-80125 Naples, Italy
Recommended Citation
GB/T 7714
Li, M,Zuo, WW,Ricciardulli, AG,et al. Embedded Nickel-Mesh Transparent Electrodes for Highly Efficient and Mechanically Stable Flexible Perovskite Photovoltaics: Toward a Portable Mobile Energy Source[J]. ADVANCED MATERIALS,2020,32(38):-.
APA Li, M.,Zuo, WW.,Ricciardulli, AG.,Yang, YG.,Liu, YH.,...&Wang, ZK.(2020).Embedded Nickel-Mesh Transparent Electrodes for Highly Efficient and Mechanically Stable Flexible Perovskite Photovoltaics: Toward a Portable Mobile Energy Source.ADVANCED MATERIALS,32(38),-.
MLA Li, M,et al."Embedded Nickel-Mesh Transparent Electrodes for Highly Efficient and Mechanically Stable Flexible Perovskite Photovoltaics: Toward a Portable Mobile Energy Source".ADVANCED MATERIALS 32.38(2020):-.
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