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Liquid-to-Solid Phase Transition of a 1,3-Dimethylimidazolium Chloride Ionic Liquid Monolayer Confined between Graphite Walls
Sha, ML(沙茂林); Wu, GZ(吴国忠); Fang, HP(方海平); Zhu, GL; Liu, YS; Wu, GZ (reprint author), Chinese Acad Sci, Shanghai Inst Appl Phys, Shanghai 201800, Peoples R China
2008
Source PublicationJOURNAL OF PHYSICAL CHEMISTRY C
ISSN1932-7447
Volume112Issue:47Pages:18584
AbstractMolecular dynamics simulations were performed to study the phase behavior of a monolayer of room temperature ionic liquid 1,3-dimethylimidazolium chloride ([Dmim][Cl]) confined between two graphite walls at 425 K. These simulations predict a first-order freezing transition from a liquid monolayer to a solid monolayer induced by varying the distance between the parallel graphite walls (H = similar to 0.65-0.95 nm). The resulting monolayer solid consisting of a hydrogen-bonded network structure is very different from bulk crystalline [Dmim][Cl]. The phase transition can be induced only at a molecular surface density of rho = 1.9/nM(2).
Subject AreaNuclear Science & Technology ; Physics
Indexed BySCI
Language英语
Funding Project应物所项目组
WOS IDWOS:000261056500044
Citation statistics
Cited Times:59[WOS]   [WOS Record]     [Related Records in WOS]
Document Type期刊论文
Identifierhttp://ir.sinap.ac.cn/handle/331007/7768
Collection中科院上海应用物理研究所2004-2010年
Corresponding AuthorWu, GZ (reprint author), Chinese Acad Sci, Shanghai Inst Appl Phys, Shanghai 201800, Peoples R China
Recommended Citation
GB/T 7714
Sha, ML,Wu, GZ,Fang, HP,et al. Liquid-to-Solid Phase Transition of a 1,3-Dimethylimidazolium Chloride Ionic Liquid Monolayer Confined between Graphite Walls[J]. JOURNAL OF PHYSICAL CHEMISTRY C,2008,112(47):18584.
APA Sha, ML,Wu, GZ,Fang, HP,Zhu, GL,Liu, YS,&Wu, GZ .(2008).Liquid-to-Solid Phase Transition of a 1,3-Dimethylimidazolium Chloride Ionic Liquid Monolayer Confined between Graphite Walls.JOURNAL OF PHYSICAL CHEMISTRY C,112(47),18584.
MLA Sha, ML,et al."Liquid-to-Solid Phase Transition of a 1,3-Dimethylimidazolium Chloride Ionic Liquid Monolayer Confined between Graphite Walls".JOURNAL OF PHYSICAL CHEMISTRY C 112.47(2008):18584.
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